That's it man, game over!
I don't foresee EVER coming across enough more and different versions of Jerry Goldsmith's U.N.C.L.E. theme or other music freatured in the show, to EVER compile another anthology. So this, the fourth one, is the last!
And here are the contents of the dead man's pockets (That's also the title of a dynamite story by Jack Finney, which may be read here.)
01. The Man from Thrush - The Clee-Shays (2:00) 1965
02. The Spy - The Guys from U.N.C.L.E. (2:31) 1966
03. Man from America (Medley: Theme from Man from U.N.C.L.E. - America) - The Ring (7:03) 1980
04. The Man from U.N.C.L.E. - The Times (5:14) 1985
05. Illya Kuryakin Looked at Me - Cleaners from Venus (2:58) 1987
06. The Man from U.N.C.L.E. - London Theatre Orchestra (2:36) 1996
07. The Man from U.N.C.L.E. - TV21 (3:24) 1998
08. The Man from U.N.C.L.E. - Johnny Pearson and His London Orchestra (2:04) 1999
09. Agent for Love - Girls from U.N.C.L.E. (2:20) 2000
10. The Man from U.N.C.L.E. - Ray Fischer (2:10) 2001
11. The Girl from U.N.C.L.E. - The Four Corners (1:41) 2001
12. Lament for a Trapped Spy - The Moon-Rays (2:14) 2002
13. Run Spy Run - The Moon-Rays (2:03) 2002
14. The Man from U.N.C.L.E. - Spy-Fi (2:05) 2003
15. Illya Kuryakin Looked at Me (Slow Version) - Cleaners from Venus (2:52) 2004
16. The Man from Thrush - Jet Set Sweden (3:54) 2005
17. The Man from U.N.C.L.E. - Los Tortures (1:40) 2005
18. The Man from U.N.C.L.E. - Paul Brooks (2:44) 2005
19. Illya Kuryakin Looked at Me - The Jennifers (3:02) 2006
20. The Man from U.N.C.L.E. - Warren Barker Orchestra (2:44) 2006
21. The Man from U.N.C.L.E. - The Countdown (2:31) 2007
22. The Man from Thrush - Movie Sounds Unlimited (2:37) 2008
23. The Man from U.N.C.L.E. - Chris Rime (featuring Lionel Fortin) (4:56) 2011
24. Napoleon Solo - George Zhen (4:44) 2011
25. Season 1 Theme - Dominik Hauser (1:07) 2012
26. Season 3 Theme - Dominik Hauser (0:41) 2012
27. The Man from U.N.C.L.E. - The Grave (2:59) 2012
28. The Man from U.N.C.L.E. - West Hell 5 (2:40) 2012
So, for other obsessive completists like me, here's something else to tide you over until the remake movie comes out.
Also included is a PDF of notes and brief commentary.
UPDATED LINK, SEPTEMBER 2015:
We wish to thank the United Network Command for Law and Enforcement, without whose assistance this compilation would not have been possible.